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Unleashing Perovskites’ Potential for Solar Fabrics

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Unleashing perovskites’ potential for solar cells

David L. Chandler | MIT News Office
February 7, 2019

Perovskites — a broad category of compounds that share a certain crystal structure — have attracted a great deal of attention as potential new solar-cell materials because of their low cost, flexibility, and relatively easy manufacturing process. But much remains unknown about the details of their structure and the effects of substituting different metals or other elements within the material.

Conventional solar cells made of silicon must be processed at temperatures above 1,400 degrees Celsius, using expensive equipment that limits their potential for production scaleup. In contrast, perovskites can be processed in a liquid solution at temperatures as low as 100 degrees, using inexpensive equipment. What’s more, perovskites can be deposited on a variety of substrates, including flexible plastics, enabling a variety of new uses that would be impossible with thicker, stiffer silicon wafers.

Now, researchers have been able to decipher a key aspect of the behavior of perovskites made with different formulations: With certain additives there is a kind of “sweet spot” where greater amounts will enhance performance and beyond which further amounts begin to degrade it. The findings are detailed this week in the journal Science, in a paper by former MIT postdoc Juan-Pablo Correa-Baena, MIT professors Tonio Buonassisi and Moungi Bawendi, and 18 others at MIT, the University of California at San Diego, and other institutions.

Perovskites are a family of compounds that share a three-part crystal structure. Each part can be made from any of a number of different elements or compounds — leading to a very broad range of possible formulations. Buonassisi compares designing a new perovskite to ordering from a menu, picking one (or more) from each of column A, column B, and (by convention) column X. “You can mix and match,” he says, but until now all the variations could only be studied by trial and error, since researchers had no basic understanding of what was going on in the material.

In previous research by a team from the Swiss École Polytechnique Fédérale de Lausanne, in which Correa-Baena participated, had found that adding certain alkali metals to the perovskite mix could improve the material’s efficiency at converting solar energy to electricity, from about 19 percent to about 22 percent. But at the time there was no explanation for this improvement, and no understanding of exactly what these metals were doing inside the compound. “Very little was known about how the microstructure affects the performance,” Buonassisi says.

Now, detailed mapping using high-resolution synchrotron nano-X-ray fluorescence measurements, which can probe the material with a beam just one-thousandth the width of a hair, has revealed the details of the process, with potential clues for how to improve the material’s performance even further.

It turns out that adding these alkali metals, such as cesium or rubidium, to the perovskite compound helps some of the other constituents to mix together more smoothly. As the team describes it, these additives help to “homogenize” the mixture, making it conduct electricity more easily and thus improving its efficiency as a solar cell. But, they found, that only works up to a certain point. Beyond a certain concentration, these added metals clump together, forming regions that interfere with the material’s conductivity and partly counteract the initial advantage. In between, for any given formulation of these complex compounds, is the sweet spot that provides the best performance, they found.

“It’s a big finding,” says Correa-Baena, who in January became an assistant professor of materials science and engineering at Georgia Tech. What the researchers found, after about three years of work at MIT and with collaborators at UCSD, was “what happens when you add those alkali metals, and why the performance improves.” They were able to directly observe the changes in the composition of the material, and reveal, among other things, these countervailing effects of homogenizing and clumping.

“The idea is that, based on these findings, we now know we should be looking into similar systems, in terms of adding alkali metals or other metals,” or varying other parts of the recipe, Correa-Baena says. While perovskites can have major benefits over conventional silicon solar cells, especially in terms of the low cost of setting up factories to produce them, they still require further work to boost their overall efficiency and improve their longevity, which lags significantly behind that of silicon cells.

Although the researchers have clarified the structural changes that take place in the perovskite material when adding different metals, and the resulting changes in performance, “we still don’t understand the chemistry behind this,” Correa-Baena says. That’s the subject of ongoing research by the team. The theoretical maximum efficiency of these perovskite solar cells is about 31 percent, according to Correa-Baena, and the best performance to date is around 23 percent, so there remains a significant margin for potential improvement.

Although it may take years for perovskites to realize their full potential, at least two companies are already in the process of setting up production lines, and they expect to begin selling their first modules within the next year or so. Some of these are small, transparent and colorful solar cells designed to be integrated into a building’s façade. “It’s already happening,” Correa-Baena says, “but there’s still work to do in making these more durable.”

Once issues of large-scale manufacturability, efficiency, and durability are addressed, Buonassisi says, perovskites could become a major player in the renewable energy industry. “If they succeed in making sustainable, high-efficiency modules while preserving the low cost of the manufacturing, that could be game-changing,” he says. “It could allow expansion of solar power much faster than we’ve seen.”

Perovskite solar cells “are now primary candidates for commercialization. Thus, providing deeper insights, as done in this work, contributes to future development,” says Michael Saliba, a senior researcher on the physics of soft matter at the University of Fribourg, Switzerland, who was not involved in this research.

Saliba adds, “This is great work that is shedding light on some of the most investigated materials. The use of synchrotron-based, novel techniques in combination with novel material engineering is of the highest quality, and is deserving of appearing in such a high-ranking journal.” He adds that work in this field “is rapidly progressing. Thus, having more detailed knowledge will be important for addressing future engineering challenges.”

The study, which included researchers at Purdue University and Argonne National Laboratory, in addition to those at MIT and UCSD, was supported by the U.S. Department of Energy, the National Science Foundation, the Skolkovo Institute of Science and Technology, and the California Energy Commission.

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  67. If you loved camping outdoors like a little one, then you can continue to enjoy it as an grown-up. With good information, and several improve preparation, it can still be an incredibly enjoyable and gratifying experience. You can find some suggestions on this page to help you. A good multi-function resource needs to be element of your outdoor camping gear. There are two forms to bring. Very first is the saw/hammer/axe 3-in-1 instrument to use for fire wood and also other work. Another is definitely the regular multiple-objective resource with many different instruments upon it like a can opener, tweezers, scissors, as well as a knife. Like a good manners for some other hikers, don’t leave your illumination on over night, should you be in close proximity to other individuals. Load a timer that you could attach to your lighting that will immediately closed them off of after having a certain time. Making lighting fixtures on overnight is a well-known problem amid most American citizen outdoorsmen! Acquire only photographs and then leave only footprints. That is the guideline when camping out. Just use the natural sources that you desire and never depart any remnants that you simply were actually camping if you abandon. Get all rubbish, extinguish and cover any fire pits, bury all human being waste, to make the spot that you camped appear just as it performed if you found it. Discover your brand new items before going outdoor camping. The exercise does truly aid. No one wants to get to the campground, only to realize which they don’t know how to use something or setup their particular tent. Training with the new gear prior to ever established feet around the camping site. Creating a fantastic outdoor camping encounter will not be hard, but you will have to take a couple of steps and make sure you keep in mind some things. Permit the ideas in the following paragraphs enable you to keep important things in your mind, to help you have a good time. Maintain understanding camping out in order to create a unforgettable practical experience every time.

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  73. When accomplished nicely, outdoor camping is amid life’s accurate pleasures. Before embarking on an outdoor experience by yourself or with family and friends, it is essential to familiarize yourself with tried and tested camping outdoors tips and advice. The content that follows offers just the commence any burgeoning in the open air enthusiast should program their next trip. An excellent multiple-function resource must be a part of your camping out items. The two main types to take. First is definitely the discovered/hammer/axe 3-in-1 instrument for firewood and other tasks. Other may be the normal multi-purpose resource with a number of instruments on it similar to a can opener, tweezers, scissors, along with a knife. Figure out your products prior to going camping out. The exercise does really help. No one wants to arrive at the camping site, only to find they don’t learn how to use some thing or put in place their particular tent. Practice with the new equipment before you at any time establish feet in the camping area. For those who have kids camping outdoors together with you, load up several craft products. When investing in to the site, demonstrate to them how you can do leaf rubbings. You will always find many different results in in all of the styles and sizes, so striving every one of them out will take time. The children will probably be pleased and you will definitely possess some peacefulness and tranquil when you loosen up and watch them. Get only images by leaving only footprints. Which is the general guideline when outdoor camping. Use only natural sources that you require and do not depart any remnants which you were actually outdoor camping whenever you abandon. Pick-up all trash can, extinguish and deal with any flame pits, bury all human being waste, making the location that you camped appear just as it managed when you found it. Knowing more details on camping, it is possible to definitely unwind and enjoy yourself once you set off into mother nature. As with any activity, the greater you realize, the greater effective your outdoor camping travels will probably be. Keep in mind the ideas you may have read through in this article to be able to get pleasure from all of your current camping out trips.

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  75. There is a reason why camping outdoors is certainly a favorite action. The fresh air and natural beauty are unrivaled. If you would like to have the joys of camping for yourself, the tips presented on this page offers you the guidance you need. You don’t really need to be a son scout to be prepared, if you plan to go camping out. One of the primary regulations is usually to be sure to explain to another person in which you may be. If there isn’t an exact spot to give, then give a common notion of major roadways close by and even Gps system coordinates if you know them and provide a timeframe of if you decide to come back. To enhance your slumbering practical experience although camping outdoors, bring a pad alongside that you could place under your sleeping bag. This pad works as a barrier in between you and also hard soil in which twigs and shrub knots might cause odd slumbering conditions. When a pad isn’t helpful, deliver a couple of more comforters you could retract more than on their selves to create some cushioning. Before leaving on the getaway, utilize your back garden to help you figure out the kinks with your camping devices. Build your tent to make sure you know (or remember!) the best way to input it up. This will also enable you to see if anything needs to be patched up. It will ensure it is much easier for you when you get towards the campsite. When proceeding outdoor camping, try and acquire low-perishable items to eat. You can find no fridges from the crazy, so anything you deliver should be held in great order. You are able to undoubtedly take a chillier to place meals in, nevertheless the cooler will probably be added bulk in your journey. As a result, make an attempt to bring a lot more no-perishable foods than perishable. Take some plastic material totes or canisters along with you when you are camping outdoors to help you retail store any food items items you may have opened up. This may always keep any creatures from swarming close to your campsite and this will also always keep different animals from getting interested in anything you possess in there. This article has offered you with plenty of great understanding about how to get the most from your camping encounter. It’s good to learn that you have the option to experience on your own having a great camping out encounter if you want to allocate the time to achieve this, so just go and practice it.

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